Published December 1994 | Version v1
Journal article

At-temperature neutron diffraction investigation of the aging process in magnesia-partially-stabilized zirconia

  • 1. Univ. of Technology, Sydney (Australia)
  • 2. Australian Nuclear Science and Technology Organization, Menai (Australia)
  • 3. Rutherford Appleton Lab., Chilton (United Kingdom). ISIS Facility

Description

A time-resolved neutron powder diffraction technique has been used to follow the changes occurring during the aging of magnesia-partially-stabilized zirconia at 1,100 C. Through quantitative phase analyses it has been possible to follow the development with aging time of tetragonal zirconia and of the δ-phase (Mg2Zr5O12, related to cubic, but with ordered anion vacancies), both at the expense of cubic zirconia. Changes in lattice parameters have been attributed to the expulsion of MgO stabilizer from the tetragonal zirconia precipitates as the aging proceeds. The broadening of peaks in the neutron diffraction pattern suggests there is considerable strain in the tetragonal precipitates in the c-direction, which is the short dimension in these lenticular precipitates. On cooling, there is some transformation of tetragonal zirconia to the monoclinic and orthorhombic phases

Additional details

Publishing Information

Journal Title
Journal of the American Ceramic Society
Journal Volume
77
Journal Issue
12
Journal Page Range
p. 3073-3076.
ISSN
0002-7820
CODEN
JACTAW