Published March 15, 2019
| Version v1
Journal article
A UO2-based salt target for rapid isolation of fission products
- 1. University of Nevada – Las Vegas, Department of Chemistry and Biochemistry (United States)
- 2. Los Alamos National Laboratory, Chemistry Division (United States)
Description
We report here an initial isolation study based upon the use of small uranium oxide particles dispersed in a soluble salt matrix to evaluate the relative recovery of fission products into acidic media. We further show that the macrostructures of the uranium microparticles are largely preserved, such that the bulk target material could be retained for additional irradiations or characterizations. Through this approach, fission products can be separated from the actinide-based target using low molarities of acid without the need to dissolve the actinide itself, reducing the amount of acidic waste. Extraction yields using two molarities of HCl and HNO3 are compared.
Additional details
Identifiers
Publishing Information
- Journal Title
- Journal of Radioanalytical and Nuclear Chemistry
- Journal Volume
- 319
- Journal Issue
- 3
- Journal Page Range
- p. 1291-1300
- ISSN
- 0236-5731
- CODEN
- JRNCDM
INIS
- Country of Publication
- Hungary
- Country of Input or Organization
- International Atomic Energy Agency (IAEA)
- INIS RN
- 54121742
- Subject category
- S38: RADIATION CHEMISTRY, RADIOCHEMISTRY AND NUCLEAR CHEMISTRY;
- Descriptors DEI
- COMPARATIVE EVALUATIONS; EXTRACTION; FISSION; FISSION PRODUCTS; HYDROCHLORIC ACID; IRRADIATION; NITRIC ACID; PARTICLES; SALTS; URANIUM; URANIUM DIOXIDE; WASTES
- Descriptors DEC
- ACTINIDE COMPOUNDS; ACTINIDES; CHALCOGENIDES; CHLORINE COMPOUNDS; ELEMENTS; EVALUATION; HALOGEN COMPOUNDS; HYDROGEN COMPOUNDS; INORGANIC ACIDS; INORGANIC COMPOUNDS; ISOTOPES; MATERIALS; METALS; NITROGEN COMPOUNDS; NUCLEAR REACTIONS; OXIDES; OXYGEN COMPOUNDS; RADIOACTIVE MATERIALS; SEPARATION PROCESSES; URANIUM COMPOUNDS; URANIUM OXIDES
Optional Information
- Copyright
- Copyright (c) 2019 Akad#Latin Small Letter E With Acute#miai Kiad#Latin Small Letter O With Acute#, Budapest, Hungary