Production of gaseous radiotracers for industrial applications

This paper describes prerequisite tests, analysis and the procedure for irradiation of gaseous targets and production of gaseous radioisotopes i.e. argon-41 (⁴¹Ar) and krypton-79 (⁷⁹Kr) in a 100 MW_Th DHRUVA reactor located at Bhabha Atomic Research Center (BARC), Trombay, Mumbai, India. The produced radioisotopes will be used as radiotracers for tracing gas phase in industrial process systems. Various details and prequalification tests required for irradiation of gaseous targets are discussed. The procedure for regular production of ⁴¹Ar and ⁷⁹Kr, and assay of their activity were standardized. Theoretically estimated and experimentally produced amounts of activities of the two radioisotopes, irradiated at identical conditions, were compared and found to be in good agreement. Based on the various tests, radiological safety analysis and standardization of the irradiation procedure, necessary approval was obtained from the competent reactor operating and safety authorities for regular production of gaseous radiotracers in DHRUVA reactor. - Highlights: • Various prerequisite tests for irradiation of gaseous targets were performed. • Procedure for production of gaseous radioisotopes was standardized. • Detailed radiological safety analysis was carried out. • Necessary approvals for production of gaseous radioisotopes were obtained. • Production of gaseous radioisotopes began in DHRUVA reactor at Trombay, Mumbai, India.