Attosecond photoelectron interference in the separable Coulomb-Volkov continuum
- 1. Laboratoire de Chimie Theorique, Faculte des Sciences, Universite de Sherbrooke, Sherbrooke, QC J1K 2R1 (Canada)
- 2. National Research Council of Canada, Ottawa, ON K1A 0R6 (Canada)
Description
We develop a description of laser-assisted x-ray photoionization based on a sudden approximation approach. By splitting the system evolution into three time stages we find necessary and sufficient conditions for spatial and temporal separation of Coulomb and Volkov continuum solutions. Using the separable Coulomb-Volkov wavefunction we present an analytical non-relativistic quantum theory of attosecond photoionization. It applies for arbitrary x-ray parameters, with both Coulomb continuum and laser field treated non-perturbatively. The theory provides a firm basis for characterizing photoelectron phase and atomic and molecular wavefunctions, by extracting them from experimental data. Using the molecular hydrogen ion as a test case, we display a variety of photoelectron interference sources in energy- and angular-resolved spectra for different pulse durations, chirps and delay times between x-ray pulse replicas. (fast track communication)
Additional details
Identifiers
- DOI
- 10.1088/0953-4075/40/5/F03;
- PII
- S0953-4075(07)39333-4;
Publishing Information
- Journal Title
- Journal of Physics. B, Atomic, Molecular and Optical Physics
- Journal Volume
- 40
- Journal Issue
- 5
- Journal Page Range
- p. F93-F103
- ISSN
- 0953-4075
- CODEN
- JPAPEH
INIS
- Country of Publication
- United Kingdom
- Country of Input or Organization
- International Atomic Energy Agency (IAEA)
- INIS RN
- 38069341
- Subject category
- S74: ATOMIC AND MOLECULAR PHYSICS;
- Descriptors DEI
- COULOMB FIELD; HYDROGEN IONS; INTERFERENCE; LASER RADIATION; MATHEMATICAL SOLUTIONS; MOLECULAR IONS; PHOTOELECTRIC EMISSION; PHOTOIONIZATION; PULSES; RELATIVISTIC RANGE; SUDDEN APPROXIMATION; WAVE FUNCTIONS; X RADIATION
- Descriptors DEC
- APPROXIMATIONS; CALCULATION METHODS; CHARGED PARTICLES; ELECTRIC FIELDS; ELECTROMAGNETIC RADIATION; ELECTRON EMISSION; EMISSION; ENERGY RANGE; FUNCTIONS; IONIZATION; IONIZING RADIATIONS; IONS; PHOTOELECTRIC EFFECT; RADIATIONS