Published November 1997 | Version v1
Journal article

Controlling the Branching Ratio of Photoionization Products under Two-Color Excitation: Competition between ac Stark Splitting and Two-Path Interference

  • 1. The Institute of Physical and Chemical Research (RIKEN), 2-1 Hirosawa, Wako, Saitama, 351-01 (Japan)
  • 2. Max-Planck-Institut fuer Quantenoptik, 85748 Garching (Germany)
  • 3. F.O.R.TH., Institute of Electronic Structure and Laser and Department of Physics, University of Crete, P.O. Box 1527, Heraklion 711 10, Crete (Greece)

Description

We investigate the variation of the photoionization yields into different ionic channels by means of the one-photon-near-resonant two-photon ionization scheme under two-color excitation. We present a general formulation and the results of specific calculations pertaining to the Ca atom with realistic parameters. A significant change of the ionization into Ca+ 4s , 3d , and 4p channels has been observed as a detuning is varied, which agrees qualitatively well with the observation by Wang, Chen, and Elliott [Phys.Rev.Lett.77, 2416 (1996)] for the Ba atom. The importance of the laser intensity effects is also addressed. copyright 1997 The American Physical Society

Additional details

Publishing Information

Journal Title
Physical Review Letters
Journal Volume
79
Journal Issue
18
Journal Page Range
p. 3367-3370.
ISSN
0031-9007
CODEN
PRLTAO

INIS

Country of Publication
United States
Country of Input or Organization
United States
INIS RN
29010931
Subject category
S74: ATOMIC AND MOLECULAR PHYSICS;
Descriptors DEI
BRANCHING RATIO; CALCIUM; DENSITY MATRIX; EXCITATION; INTERFERENCE; IONIZATION; NUMERICAL ANALYSIS; PHOTOIONIZATION; STARK EFFECT; TIME DEPENDENCE
Descriptors DEC
ALKALINE EARTH METALS; ELEMENTS; ENERGY-LEVEL TRANSITIONS; MATHEMATICS; MATRICES; METALS