Published April 22, 2005 | Version v1
Journal article

Efficient and long-lived field-free orientation of molecules by a single hybrid short pulse

  • 1. Center for Nonlinear Phenomena and Complex Systems, Universite Libre de Bruxelles, 1050 Brussels (Belgium)
  • 2. Laboratoire de Physique de l'Universite de Bourgogne, UMR CNRS 5027, BP 47870, 21078 Dijon (France)

Description

We show that a combination of a half-cycle pulse and a short nonresonant laser pulse produces a strongly enhanced postpulse orientation. Robust transients that display both efficient and long-lived orientation are obtained. The mechanism is analyzed in terms of optimal oriented target states in finite Hilbert subspaces and shows that hybrid pulses can prove useful for other control issues

Additional details

Publishing Information

Journal Title
Physical Review Letters
Journal Volume
94
Journal Issue
15
Journal Page Range
p. 153003-153003.4
ISSN
0031-9007
CODEN
PRLTAO

INIS

Country of Publication
United States
Country of Input or Organization
International Atomic Energy Agency (IAEA)
INIS RN
36069217
Subject category
S71: CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS;
Descriptors DEI
CONTROL; LASERS; ORIENTATION; PHOTON-MOLECULE COLLISIONS; PULSES; RADIATION PRESSURE; TRANSIENTS
Descriptors DEC
COLLISIONS; MOLECULE COLLISIONS; PHOTON COLLISIONS

Optional Information

Notes
(c) 2005 The American Physical Society