Published January 1, 2013 | Version v1
Journal article

Spherical analyzers and monochromators for resonant inelastic hard X-ray scattering: a compilation of crystals and reflections

  • 1. Advanced Photon Source, Argonne National Laboratory, 9700 South Cass Avenue, Argonne, IL 60439 (United States)

Description

Resonant inelastic X-ray scattering (RIXS) experiments require special sets of near-backscattering spherical diced analyzers and high-resolution monochromators for every distinct absorption-edge energy or emission line. For the purpose of aiding the design and planning of efficient RIXS experiments, a compilation of suitable crystal materials and viable reflections for hard X-rays, together with energy resolution and throughput information, is presented. Resonant inelastic X-ray scattering (RIXS) experiments require special sets of near-backscattering spherical diced analyzers and high-resolution monochromators for every distinct absorption-edge energy and emission line. For the purpose of aiding the design and planning of efficient RIXS experiments, comprehensive lists of suitable analyzer reflections for silicon, germanium, α-quartz, sapphire and lithium niobate crystals were compiled for a multitude of absorption edges and emission lines. Analyzers made from lithium niobate, sapphire or α-quartz offer many choices of reflections with intrinsic resolutions currently unattainable from silicon or germanium. In some cases these materials offer higher intensities at comparable resolutions. While lithium niobate, sapphire or α-quartz analyzers are still in an early stage of development, the present compilation can serve as a computational basis for assessing expected and actual performance. With regard to high-resolution monochromators, bandpass and throughput calculations for combinations of double-crystal, high-heat-load and near-backscattering high-resolution channel-cuts were assembled. The compilation of these analyzer and monochromator data is publicly available on a website

Availability note (English)

Available from http://dx.doi.org/10.1107/S0909049512043154; Available from http://www.ncbi.nlm.nih.gov/pmc/articles/PMC3943536

Additional details

Publishing Information

Journal Title
Journal of Synchrotron Radiation
Journal Volume
20
Journal Issue
Pt 1
Journal Page Range
p. 74-79
ISSN
0909-0495
CODEN
JSYRES

Optional Information

Copyright
Copyright (c) Thomas Gog et al. 2013
Notes
PMCID: PMC3943536; PMID: 23254658; PUBLISHER-ID: ie5087; OAI: oai:pubmedcentral.nih.gov:3943536; This is an open-access article distributed under the terms of the Creative Commons Attribution Licence, which permits unrestricted use, distribution, and reproduction in any medium, provided the original authors and source are cited.