Final design for thermal epithermal experiments (TEX) with ZPPR plutonium/aluminium plates with polyethylene and tantalum - 13592

Lawrence Livermore National Laboratory has completed the final design for the first phase of the Thermal Epithermal experiments (TEX), which focused on critical configurations composed of plutonium/aluminum Zero Power Physics Reactor (ZPPR) plates moderated by polyethylene with and without a tantalum diluent. ²³⁹Pu and ²⁴⁰Pu were identified as being the number one and two nuclear data need by the nuclear criticality safety and nuclear data communities, with special emphasis placed on performance issues of the Pu cross sections in the intermediate energy region. Preliminary TEX design recommended tantalum as the first diluent to pursue for final design, as it represented a high priority data need, showed the highest sensitivity and largest contribution to uncertainty with the Pu ZPPR system, and a large number of high quality Ta plates from the ZPPR inventory in Idaho was readily available. The goals of the new critical experiments are 1) to create assemblies that span a wide range of fission energy spectra, from thermal (below 0.625 eV), through the intermediate (0.65 eV to 100 keV), and to fast energies (above 100 keV), and 2) to easily modify the assemblies to include high priority materials like tantalum. A total of ten critical configurations were designed as part of CED-2. Five TEX experiments (Experiments 1-5) were designed to establish baseline configurations with the Pu ZPPR plates covering the thermal, intermediate, and fast fission energy regimes. For all five experiments, the ZPPR plates will be arranged in layers of 24 plates (6 plates by 4 plates), resulting in approximately a 12 inch by 12 inch footprint. Multiple layers will be stacked together with varying thicknesses of interspersed polyethylene placed between the layers to fine tune the neutron spectrum of the assembly. The other five experiments (Experiments 6-10) will be similar to the five baseline experiments, except that a tantalum layer will be placed next to each plutonium plate layer, thus diluting the stack and allowing for tests of the neutron cross section for tantalum. (authors)