Published August 7, 2024 | Version v1
Journal article

Metamagnetism and anomalous magnetotransport properties in rare-earth-based polar semimetals RAuGe (R=Dy, Ho, and Gd)

  • 1. Division of Physics, Mathematics and Astronomy, California Institute of Technology, Pasadena, California 91125, USA
  • 2. Department of Advanced Materials Science, University of Tokyo, Kashiwa 277-8561, Japan
  • 3. RIKEN Center for Emergent Matter Science (CEMS), Wako 351-0198, Japan

Description

We report the magnetic, magnetoelastic, and magnetotransport properties of single crystals of polar magnets RAuGe (R=Dy, Ho, and Gd), grown by Au-Ge self-flux. Magnetization and magnetostriction measurements reveal multistep metamagnetic transitions for the c-axis magnetic field (Hc) for DyAuGe and HoAuGe, suggesting magnetic frustration in the triangular lattice of R ions. The magnetic phase diagrams have clarified a close connection between the magnetoelastic property and the emergence of the intermediate metamagentic phase. The magnetic-field dependence of the resistivity and Hall resistivity reveal the semimetallic transport dominated by hole-type carriers, consistent with the behavior in a nonmagnetic analog YAuGe. We also identify a signature of an anomalous Hall effect (AHE) proportional to the field-induced magnetization in R=Dy, Ho, and Gd. GdAuGe shows magnetic and transport behavior as reported in a previous study using Bi-flux grown single crystals, while the self-flux grown crystal shows larger magnetoresistance (345%, at 1.8 K and 9 T) due to higher hole-type carrier mobility [6400cm2/(Vs)]. Using the two-band model analysis considering the mobility change during the magnetization process, we extract the anomalous Hall conductivity: 1200 and 530 S/cm for R=Dy and Ho, respectively, at 1.8 K with 9 T for Hc. The magnitude of conductivity suggests a contribution of intrinsic origin, possibly related to the Berry curvature in the electron bands induced by the time-reversal symmetry breaking and the polar lattice.

Additional details

Identifiers

DOI
10.1103/PhysRevB.110.064409;
arXiv
arXiv:2405.00628;
Crossref Funder ID
10.13039/501100001700; 10.13039/501100003844; 10.13039/501100001691; 10.13039/501100004721;

Publishing Information

Journal Title
Physical Review B
Journal Volume
110
Journal Issue
6
Journal Page Range
11 pgs.
ISSN
1550-235X

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