Published May 1993 | Version v1
Journal article

Laser-induced stabilization and trapping andhardening in intense laser fields

Description

We study the intensity-dependent behavior of laser-induced vibrational quasi-energy (VQE) resonance structure and photodissociation rates of H2+ molecular ions in intense laser fields and report a novel new high-intensity phenomenon. At strong fields, the vibrational levels are shifted and broadened and break into several separate VQE resonance groups. Distortion of the internuclear potential by the fields leads to the formation of various (field-dressed) adiabatic potential wells near multiphoton resonances which can support long-lived resonance states. The most striking finding is that high-lying VQE resonance states can in fact become more stabilized and longer lived at higher laser intensities, a phenomenon which may be termed as open-quotes bond hardening.close quotes Time-dependent calculations confirm the laser-induced stabilization reveals that molecular population may be trapped simultaneously in different potential wells, at different internuclear separations

Additional details

Publishing Information

Journal Title
Bulletin of the American Physical Society
Journal Volume
38
Journal Issue
3
Journal Page Range
p. 1091.ME4.
ISSN
0003-0503
CODEN
BAPSA6

Conference

Title
1993 American Physical Society annual meeting on atomic, molecular, and topical physics.
Dates
16-19 May 1993.
Place
Reno, NV (United States).

INIS

Country of Publication
United States
Country of Input or Organization
United States
INIS RN
27078714
Subject category
S74: ATOMIC AND MOLECULAR PHYSICS;
Resource subtype / Literary indicator
Conference
Descriptors DEI
CHEMICAL BONDS; DISSOCIATION; HYDROGEN IONS; LASER RADIATION; MOLECULAR IONS; MULTI-PHOTON PROCESSES; TRAPPING; VIBRATIONAL STATES
Descriptors DEC
CHARGED PARTICLES; ELECTROMAGNETIC RADIATION; ENERGY LEVELS; EXCITED STATES; IONS; RADIATIONS

Optional Information

Secondary number(s)
CONF-9305421--.