Laser-induced stabilization and trapping andhardening in intense laser fields
Description
We study the intensity-dependent behavior of laser-induced vibrational quasi-energy (VQE) resonance structure and photodissociation rates of H2+ molecular ions in intense laser fields and report a novel new high-intensity phenomenon. At strong fields, the vibrational levels are shifted and broadened and break into several separate VQE resonance groups. Distortion of the internuclear potential by the fields leads to the formation of various (field-dressed) adiabatic potential wells near multiphoton resonances which can support long-lived resonance states. The most striking finding is that high-lying VQE resonance states can in fact become more stabilized and longer lived at higher laser intensities, a phenomenon which may be termed as open-quotes bond hardening.close quotes Time-dependent calculations confirm the laser-induced stabilization reveals that molecular population may be trapped simultaneously in different potential wells, at different internuclear separations
Additional details
Publishing Information
- Journal Title
- Bulletin of the American Physical Society
- Journal Volume
- 38
- Journal Issue
- 3
- Journal Page Range
- p. 1091.ME4.
- ISSN
- 0003-0503
- CODEN
- BAPSA6
Conference
- Title
- 1993 American Physical Society annual meeting on atomic, molecular, and topical physics.
- Dates
- 16-19 May 1993.
- Place
- Reno, NV (United States).
INIS
- Country of Publication
- United States
- Country of Input or Organization
- United States
- INIS RN
- 27078714
- Subject category
- S74: ATOMIC AND MOLECULAR PHYSICS;
- Resource subtype / Literary indicator
- Conference
- Descriptors DEI
- CHEMICAL BONDS; DISSOCIATION; HYDROGEN IONS; LASER RADIATION; MOLECULAR IONS; MULTI-PHOTON PROCESSES; TRAPPING; VIBRATIONAL STATES
- Descriptors DEC
- CHARGED PARTICLES; ELECTROMAGNETIC RADIATION; ENERGY LEVELS; EXCITED STATES; IONS; RADIATIONS
Optional Information
- Secondary number(s)
- CONF-9305421--.