Magnetism in the axion insulator candidate
Creators
- 1. Institute for Solid State and Materials Physics, Technical University of Dresden, 01062 Dresden, Germany
- 2. Los Alamos National Laboratory, Los Alamos, New Mexico 87545, USA
- 3. Department of Physics, Durham University, South Road, Durham, DH1 3LE, United Kingdom
- 4. Memorial University, Department of Physics and Physical Oceanography, St. John's, NL, A1B 3X7, Canada
- 5. Laboratory for Muon-Spin Spectroscopy, Paul Scherrer Institute, CH-5232 Villigen, Switzerland
- 6. ISIS Facility, STFC, Rutherford Appleton Laboratory, Chilton, Didcot, Oxfordshire, OX11 0QX, United Kingdom
- 7. London Centre for Nanotechnology and Department of Physics and Astronomy, University College London, London WC1E 6BT, United Kingdom
- 8. Diamond Light Source Ltd., Didcot OX11 0DE, United Kingdom
Description
is a member of a family of orthorhombic nonsymmorphic rare-earth intermetallics that combines large localized magnetic moments and itinerant exchange with a low carrier density and perpendicular glide planes. This may result in special topological crystalline (wallpaper fermion) or axion insulating phases. Recent studies of single crystals have revealed colossal negative magnetoresistance and multiple magnetic phase transitions. Here, we clarify this ordering process using neutron scattering, resonant elastic x-ray scattering, muon spin-rotation, and magnetometry. The nonsymmorphic and multisite character of results in coplanar noncollinear magnetic structures with an Ising-like net magnetization along the axis. A reordering transition, attributable to competing ferro- and antiferromagnetic couplings, manifests as the onset of a second commensurate Fourier component. In the absence of spatially resolved probes, the experimental evidence for this low-temperature state can be interpreted either as an unusual double- structure or in a phase separation scenario. The net magnetization produces variable anisotropic hysteretic effects which also couple to charge transport. The implied potential for functional domain physics and topological transport suggests that this structural family may be a promising platform to implement concepts of topological antiferromagnetic spintronics.
Files
10.1103_PhysRevB.109.174404.pdf
Files
(2.4 MB)
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Additional details
Identifiers
- DOI
- 10.1103/PhysRevB.109.174404;
- arXiv
- arXiv:2312.15054;
- Crossref Funder ID
- 10.13039/501100005687; 10.13039/501100000271; 10.13039/501100004219; 10.13039/501100001647; 10.13039/501100001656; 10.13039/501100000266; 10.13039/100000015; 10.13039/100006151; 10.13039/501100001711; 10.13039/501100002957; 10.13039/501100001659; 10.13039/100005156;
Publishing Information
- Journal Title
- Physical Review B
- Journal Volume
- 109
- Journal Issue
- 17
- Journal Page Range
- 9 pgs.
- ISSN
- 1550-235X
INIS
- Country of Publication
- United States
- Country of Input or Organization
- International Atomic Energy Agency (IAEA)
- Subject category
- S75: CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY;
- Descriptors DEI
- ANTIFERROMAGNETISM; EXCHANGE INTERACTIONS; FERROMAGNETISM; HYSTERESIS; INTERMETALLIC COMPOUNDS; MAGNETIC MOMENTS; MAGNETIZATION; MAGNETORESISTANCE; MONOCRYSTALS; NEUTRON DIFFRACTION; ORTHORHOMBIC LATTICES; PHASE TRANSFORMATIONS; RARE EARTHS; ROTATION; TOPOLOGY; X-RAY DIFFRACTION
- Descriptors DEC
- ALLOYS; COHERENT SCATTERING; CRYSTAL LATTICES; CRYSTAL STRUCTURE; CRYSTALS; DIFFRACTION; ELECTRIC CONDUCTIVITY; ELECTRICAL PROPERTIES; ELEMENTS; INTERACTIONS; MAGNETISM; MATHEMATICS; METALS; MOTION; PHYSICAL PROPERTIES; SCATTERING; THREE-DIMENSIONAL LATTICES
Optional Information
- Contract/Grant/Project number
- I-20190272; I-20210419; EP/N032128/1; EP/N027671/1; EP/N034694/1; 200650; 247310070; 501391385
- Notes
- Contact Email: marein.rahn@tu-dresden.de; Contact Email: marc.janoschek@psi.ch; Record automatically processed
- Funding organization
- Goethe-Universität Frankfurt am Main; Science and Technology Facilities Council; Paul Scherrer Institut; Deutsches Elektronen-Synchrotron; Helmholtz-Gemeinschaft; Engineering and Physical Sciences Research Council; U.S. Department of Energy; Basic Energy Sciences; Schweizerischer Nationalfonds zur Förderung der Wissenschaftlichen Forschung; Technische Universität Dresden; Deutsche Forschungsgemeinschaft; Alexander von Humboldt-Stiftung