Published May 2, 2024 | Version v1
Journal article Open

Magnetism in the axion insulator candidate Eu5In2Sb6

  • 1. Institute for Solid State and Materials Physics, Technical University of Dresden, 01062 Dresden, Germany
  • 2. Los Alamos National Laboratory, Los Alamos, New Mexico 87545, USA
  • 3. Department of Physics, Durham University, South Road, Durham, DH1 3LE, United Kingdom
  • 4. Memorial University, Department of Physics and Physical Oceanography, St. John's, NL, A1B 3X7, Canada
  • 5. Laboratory for Muon-Spin Spectroscopy, Paul Scherrer Institute, CH-5232 Villigen, Switzerland
  • 6. ISIS Facility, STFC, Rutherford Appleton Laboratory, Chilton, Didcot, Oxfordshire, OX11 0QX, United Kingdom
  • 7. London Centre for Nanotechnology and Department of Physics and Astronomy, University College London, London WC1E 6BT, United Kingdom
  • 8. Diamond Light Source Ltd., Didcot OX11 0DE, United Kingdom

Description

Eu5In2Sb6 is a member of a family of orthorhombic nonsymmorphic rare-earth intermetallics that combines large localized magnetic moments and itinerant exchange with a low carrier density and perpendicular glide planes. This may result in special topological crystalline (wallpaper fermion) or axion insulating phases. Recent studies of Eu5In2Sb6 single crystals have revealed colossal negative magnetoresistance and multiple magnetic phase transitions. Here, we clarify this ordering process using neutron scattering, resonant elastic x-ray scattering, muon spin-rotation, and magnetometry. The nonsymmorphic and multisite character of Eu5In2Sb6 results in coplanar noncollinear magnetic structures with an Ising-like net magnetization along the a axis. A reordering transition, attributable to competing ferro- and antiferromagnetic couplings, manifests as the onset of a second commensurate Fourier component. In the absence of spatially resolved probes, the experimental evidence for this low-temperature state can be interpreted either as an unusual double-q structure or in a phase separation scenario. The net magnetization produces variable anisotropic hysteretic effects which also couple to charge transport. The implied potential for functional domain physics and topological transport suggests that this structural family may be a promising platform to implement concepts of topological antiferromagnetic spintronics.

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10.1103_PhysRevB.109.174404.pdf

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Additional details

Identifiers

DOI
10.1103/PhysRevB.109.174404;
arXiv
arXiv:2312.15054;
Crossref Funder ID
10.13039/501100005687; 10.13039/501100000271; 10.13039/501100004219; 10.13039/501100001647; 10.13039/501100001656; 10.13039/501100000266; 10.13039/100000015; 10.13039/100006151; 10.13039/501100001711; 10.13039/501100002957; 10.13039/501100001659; 10.13039/100005156;

Publishing Information

Journal Title
Physical Review B
Journal Volume
109
Journal Issue
17
Journal Page Range
9 pgs.
ISSN
1550-235X