Magnetism and electronic transport in irradiated organic conductors
Description
Quasi-one-dimensional conductors are metallic in a large temperature range. The electronic gas instability can drive a phase transition at low temperature. In one-dimensional conditions, precursor fluctuations grow in the high temperature regime and can give a collective current transport. Under irradiation the quasi-one-dimensional electrons are localized and the conductivity becomes typical of a phonon assisted tunneling between metallic particles. In this study we describe the magnetism of this localized electrons. This disorder reduces the interaction between electronic spins and phonons and favours the interaction between localized spins. But if the electronic gas is less one-dimensional, irradiation disorder can not localize electrons. Our conductivity measurements prove that the disorder first reduces the electronic relaxation before induces the above mentioned localization. Moreover the fluctuative conductivity is revealed by irradiation thanks to a discrepancy with respect to one-electron model. TTF-TCNQ and (TMTSF)2ClO4 are investigated in that way
Availability note (English)
MF available from INIS under the Report Number.Abstract (French)
Les conducteurs organiques presentent un large domaine de temperature dans lequel ils sont metalliques. L'instabilite de leur gaz electronique, tres anisotrope, peut conduire a une transition de phase a basse temperature. Mais, si les electrons sont suffisamment unidimensionnels, des fluctuations annoncant cette instabilite se developpent dans le regime haute temperature et peuvent donner un transport collectif du courant. Les defauts crees par irradiation sont capables de localiser les electrons presque unidimensionnels. La conductivite devient sous irradiation caracteristique d'un effet tunnel assiste par les phonons entre particules metalliques. Cette etude decrit le magnetisme de ces electrons. Le desordre reduit l'interaction des spins electroniques avec les phonons et augmente celle entre les spins localises. Mais si le gaz electronique n'est plus suffisamment unidimensionnel le desordre d'irradiation ne peut plus localiser les electrons. Notre etude de conductivite montre que le desordre diminue d'abord le temps de relaxation electronique avant d'induire a partir d'une certaine dose la localisation precedemment decrite. En outre, la conductivite collective peut etre mise en evidence par l'irradiation grace aux ecarts de comportement par rapport au modele a un electron. TTFx - TCNQ et (TMTSF)2ClO4 sont etudies de ce point de vueFiles
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Additional details
Additional titles
- Original title (French)
- Magnetisme et transport electronique dans les conducteurs organiques irradies
Publishing Information
- Imprint Pagination
- 168 p.
- Report number
- CEA-R--5335
INIS
- Country of Publication
- France
- Country of Input or Organization
- France
- INIS RN
- 17039089
- Subject category
- S36: MATERIALS SCIENCE;
- Resource subtype / Literary indicator
- Thesis
- Descriptors DEI
- CHARGE DENSITY; CYCLOALKENES; ELECTRIC CONDUCTIVITY; ELECTRON SPIN RESONANCE; ELECTRONS; HEAVY IONS; ONE-DIMENSIONAL CALCULATIONS; PHYSICAL RADIATION EFFECTS; SPIN-LATTICE RELAXATION; SPIN-SPIN RELAXATION; TMTSF
- Descriptors DEC
- ALKENES; CHARGED PARTICLES; ELECTRICAL PROPERTIES; ELEMENTARY PARTICLES; FERMIONS; HETEROCYCLIC COMPOUNDS; HYDROCARBONS; IONS; LEPTONS; MAGNETIC RESONANCE; ORGANIC COMPOUNDS; PHYSICAL PROPERTIES; RADIATION EFFECTS; RELAXATION; RESONANCE; SELENIUM COMPOUNDS