Published February 21, 2024 | Version v1
Journal article

Optical drive of amplitude and phase modes in excitonic insulators

  • 1. Department of Physics, Sharif University of Technology, Tehran 14588-89694, Iran

Description

Motivated by recent interest in exploring excitonic condensate as the ground state of some narrow-band-gap semiconductors, such as transition metal dichalcogenides and layered chalcogenide material Ta2NiSe5, in this paper, we theoretically study the dynamics of condensate in response to periodically driven laser fields with different polarizations and intensities. In particular, we consider laser light beams with bicircular and circular polarizations breaking the time-reversal symmetry, and linear polarization. We show that the amplitude of the condensate oscillates in time during irradiating by light with a magnitude depending on the light intensity. The dynamics survives even after the light is switched off. The phase mode, however, changes linearly with time for a condensate originating from purely electronic correlations. We further show that in the presence of electron-phonon coupling, the linear-in-time behavior is replaced by a harmonically oscillating behavior, a manifestation of gapped phase modes due to relative band charge symmetry breaking. Furthermore, we show that the primarily electronic and primarily lattice cases corresponding to strong and weak electron-phonon coupling, respectively, reveal distinct dynamics of the condensate, an observation which can modify the optical response of an excitonic insulator by stimulating amplitude and phase modes in the former case.

Additional details

Identifiers

DOI
10.1103/PhysRevB.109.075146;
arXiv
arXiv:2311.04051;
Crossref Funder ID
10.13039/501100003968;

Publishing Information

Journal Title
Physical Review B
Journal Volume
109
Journal Issue
7
Journal Page Range
13 pgs.
ISSN
1550-235X

Optional Information

Copyright
©2024 American Physical Society
Contract/Grant/Project number
4027770
Notes
Contact Email: kargarian@sharif.edu; Record automatically processed
Funding organization
Iran National Science Foundation