Published December 1, 2016 | Version v1
Journal article

Spatially and spectrally resolved quantum path interference with chirped driving pulses

  • 1. Department of Physics, Lund University, Box 118, SE-222 10 Lund (Sweden)
  • 2. Department of Chemical Physics, Lund University, Box 124, SE-222 10 Lund (Sweden)
  • 3. Louisiana State University, Baton Rouge, 70803-4001, LA (United States)

Description

We measure spectrally and spatially resolved high-order harmonics generated in argon using chirped multi-cycle laser pulses. Using a stable, high-repetition rate laser we observe detailed interference structures in the far-field. The structures are of two kinds; off-axis interference from the long trajectory only and on-axis interference including the short and long trajectories. The former is readily visible in the far-field spectrum, modulating both the spectral and spatial profile. To access the latter, we vary the chirp of the fundamental, imparting different phases on the different trajectories, thereby changing their relative phase. Using this method together with an analytical model, we are able to explain the on-axis behaviour and access the dipole phase parameters for the short ( α s ) and long ( α l ) trajectories. The extracted results compare very well with phase parameters calculated by solving the time-dependent Schrödinger equation. Going beyond the analytical model, we are also able to successfully reproduce the off-axis interference structure. (paper)

Availability note (English)

Available from http://dx.doi.org/10.1088/1367-2630/aa511f

Additional details

Identifiers

Publishing Information

Journal Title
New Journal of Physics
Journal Volume
18
Journal Issue
12
Journal Page Range
[17 p.]
ISSN
1367-2630

INIS

Country of Publication
United Kingdom
Country of Input or Organization
International Atomic Energy Agency (IAEA)
INIS RN
51033719
Subject category
S71: CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS;
Descriptors DEI
ARGON; COMPARATIVE EVALUATIONS; DIPOLES; EQUATIONS; HARMONICS; LASERS; TIME DEPENDENCE; TRAJECTORIES
Descriptors DEC
ELEMENTS; EVALUATION; FLUIDS; GASES; MULTIPOLES; NONMETALS; OSCILLATIONS; RARE GASES