The self-absorption effect of gamma rays in 239Pu

Nuclear materials assay with gamma-ray spectrum measurement is a well-established method for safeguards. However, for a thick source, the self-absorption of characteristic low-energy gamma rays has been a handicap to accurate assay. The author has carried out Monte Carlo simulations to study this effect using the 239Pu α-decay gamma-ray spectrum as an example. The thickness of a plutonium metal source can be considered a function of gamma-ray intensity ratios. In a practical application, gamma-ray intensity ratios can be obtained from a measured spectrum. With the help of calculated curves, scientists can find the source thickness and make corrections to gamma-ray intensities, which then lead to an accurate quantitative determination of radioactive isotopes in the material