Published April 1989 | Version v1
Journal article

Electronic structure of OP(NCS)3, BCl3xOP(NCS)3, and BCl3xOPCl3

  • 1. Kievskij Gosudarstvennyj Univ., Kiev (Ukrainian SSR)

Description

Calculation of geometry and electronic structure of OP(NCS)3, BCl3xOP(NCS)3, BCl3xOPCl3 and related molecules using MNDO SCF MO LCAO methods is carried out. It is shown that during complexing part of electron density transfers from ligand to BCl3 molecule. Effective negative charge of 0.565e transfers from OP(NCS)3 molecule to BCl3 and from three NCS groups - 0.592e. Atoms or groups combining with phosphorus make the main contribution to donor ability of ligands. Chemical bond characteristics, effective charges of atoms are presented. Formation enthalpy of BCl3xOP(NCS)3 is -163.55 kJ/mol

Additional details

Additional titles

Original title (Russian)
Электронное строение OP(NCS)

Publishing Information

Journal Title
Ukrainskij Khimicheskij Zhurnal
Journal Volume
55
Journal Issue
4
Series
Ukr. Khim. Zh.
Journal Page Range
351-354
ISSN
0041-6045
CODEN
UKZHA