Optimal networks for excitonic energy transport
- 1. Physikalisches Institut, Albert-Ludwigs-Universitaet Freiburg, Hermann-Herder Strasse 3, D-79104 Freiburg (Germany)
Description
We investigate coherent and incoherent excitation transfer in a random network with dipole-dipole interactions as a model system describing energy transport, e.g., in photosynthetic light-harvesting complexes or gases of cold Rydberg atoms. For this purpose, we introduce and compare two different measures (the maximum output probability and the average transfer time) for the efficiency of transport from the input to the output site. We especially focus on optimal configurations which maximize the transfer efficiency and the impact of dephasing noise on the transport dynamics. For most configurations of the random network, the transfer efficiency increases when adding noise, giving rise to essentially classical transport. These noise-assisted configurations are, however, systematically less efficient than the optimal configurations. The latter reach their highest efficiency for purely coherent dynamics, i.e. in the absence of noise.
Availability note (English)
Available from http://dx.doi.org/10.1088/0953-4075/44/18/184012Additional details
Identifiers
- DOI
- 10.1088/0953-4075/44/18/184012;
- PII
- S0953-4075(11)89803-2;
Publishing Information
- Journal Title
- Journal of Physics. B, Atomic, Molecular and Optical Physics
- Journal Volume
- 44
- Journal Issue
- 18
- Journal Page Range
- [10 p.]
- ISSN
- 0953-4075
- CODEN
- JPAPEH
INIS
- Country of Publication
- United Kingdom
- Country of Input or Organization
- International Atomic Energy Agency (IAEA)
- INIS RN
- 43012793
- Subject category
- S74: ATOMIC AND MOLECULAR PHYSICS;
- Descriptors DEI
- ATOMS; COHERENT PRODUCTION; COMPARATIVE EVALUATIONS; CONFIGURATION; DIPOLES; EFFICIENCY; ENERGY TRANSFER; EXCITATION; GASES; INTERACTIONS; NOISE; PROBABILITY; RANDOMNESS; RYDBERG STATES; TEMPERATURE RANGE 0000-0013 K; VISIBLE RADIATION
- Descriptors DEC
- ELECTROMAGNETIC RADIATION; ENERGY LEVELS; ENERGY-LEVEL TRANSITIONS; EVALUATION; EXCITED STATES; FLUIDS; INTERACTIONS; MULTIPOLES; PARTICLE INTERACTIONS; PARTICLE PRODUCTION; RADIATIONS; TEMPERATURE RANGE