Upward migration of radio-cesium and strontium in a sand-filled lysimeter

The upward migration of 134Cs, 137Cs, and 90Sr was observed in a silica sand-filled lysimeter at the Field Lysimeter Investigations: Low Level Waste Data Base Development experiment site at Oak Ridge National Laboratory. The source of the radionuclides first observed on the surface was identified from isotopic analysis as being from the buried waste. Cores of the sand were collected and analyzed for the vertical distribution of the radionuclides. Results of analyses revealed that pulses (elevated levels) in the activity of the Cs and Sr radioisotopes occurred at the same depths. During the sectioning of the sand core collected from directly above the buried waste form it was discovered that a fine root from an unidentified plant was present throughout all but the upper few centimeters of the core. Because the upward migration was unexpected, information that may lead to the determination of a definitive mechanism of migration was not preserved. The distribution of the radionuclides coupled with the presence of the root suggest that Cs and Sr migrated upward in the evapotranspiration stream of the root. Further study must be undertaken to confirm this phenomenon. Upward migration of radionuclides as observed here could result in direct exposures and offsite releases from underground storage facilities. (Copyright (c) 1998 Elsevier Science B.V., Amsterdam. All rights reserved.)