Three-dimensional investigation of ozone pollution in the lower troposphere using an unmanned aerial vehicle platform

Potential utilities of instrumented lightweight unmanned aerial vehicles (UAVs) to quickly characterize tropospheric ozone pollution and meteorological factors including air temperature and relative humidity at three-dimensional scales are highlighted in this study. Both vertical and horizontal variations of ozone within the 1000 m lower troposphere at a local area of 4 × 4 km² are investigated during summer and autumn times. Results from field measurements show that the UAV platform has a sufficient reliability and precision in capturing spatiotemporal variations of ozone and meteorological factors. The results also reveal that ozone vertical variation is mainly linked to the vertical distribution patterns of air temperature and the horizontal transport of air masses from other regions. In addition, significant horizontal variations of ozone are also observed at different levels. Without major exhaust sources, ozone horizontal variation has a strong correlation with the vertical convection intensity of air masses within the lower troposphere. Higher air temperatures are usually related to lower ozone horizontal variations at the localized area, whereas underlying surface diversity has a week influence. Three-dimensional ozone maps are obtained using an interpolation method based on UAV collected samples, which are capable of clearly demonstrating the diurnal evolution processes of ozone within the 1000 m lower troposphere. - Highlights: • A lightweight UAV platform is assessed and used to investigate ozone pollution. • Strong vertical and horizontal variations of ozone are observed within the PBL. • Air temperature has a strong correlation with ozone spatiotemporal variations. - An instrumented lightweight UAV platform in measuring ozone spatiotemporal variations is developed and validated in this study.