Published January 24, 2024 | Version v1
Journal article

Odd Nonlinear Conductivity under Spatial Inversion in Chiral Tellurium

  • 1. CIC nanoGUNE BRTA, 20018 Donostia-San Sebastián, Basque Country, Spain
  • 2. IKERBASQUE, Basque Foundation for Science, 48009 Bilbao, Basque Country, Spain
  • 3. AGH University of Krakow, Institute of Electronics, 30-059 Kraków, Poland
  • 4. Centro de Física de Materiales CSIC-UPV/EHU, 20018 Donostia-San Sebastián, Basque Country, Spain
  • 5. Donostia International Physics Center, 20018 Donostia-San Sebastián, Basque Country, Spain
  • 6. Unité Mixte de Physique, CNRS, Thales, Université Paris-Saclay, 91767 Palaiseau, France
  • 7. Department of Materials Physics UPV/EHU, 20018 Donostia-San Sebastián, Basque Country, Spain

Description

Electrical transport in noncentrosymmetric materials departs from the well-established phenomenological Ohm's law. Instead of a linear relation between current and electric field, a nonlinear conductivity emerges along specific crystallographic directions. This nonlinear transport is fundamentally related to the lack of spatial inversion symmetry. However, the experimental implications of an inversion symmetry operation on the nonlinear conductivity remain to be explored. Here, we report on a large, nonlinear conductivity in chiral tellurium. By measuring samples with opposite handedness, we demonstrate that the nonlinear transport is odd under spatial inversion. Furthermore, by applying an electrostatic gate, we modulate the nonlinear output by a factor of 300, reaching the highest reported value excluding engineered heterostructures. Our results establish chiral tellurium as an ideal compound not just to study the fundamental interplay between crystal structure, symmetry operations and nonlinear transport; but also to develop wireless rectifiers and energy-harvesting chiral devices.

Additional details

Identifiers

DOI
10.1103/PhysRevLett.132.046303;
arXiv
arXiv:2311.08267;
Crossref Funder ID
10.13039/100010434; 10.13039/501100011033; 10.13039/501100014434; 10.13039/501100003451;

Publishing Information

Journal Title
Physical Review Letters
Journal Volume
132
Journal Issue
4
Journal Page Range
7 pgs.
ISSN
0031-9007

Optional Information

Copyright
© 2024 American Physical Society
Contract/Grant/Project number
PID2021-122511OB-I00; PID2021-128760NB-I00; PID2021-129035NB-I00; CEX2020-001038-M; 100010434; LCF/BQ/DR21/11880030; RYC2021-034836-I; RYC2021-031705-I; PPN/BEK/2020/1/00118/DEC/1
Notes
Contact Email: Corresponding author: marco.gobbi@ehu.eus; Contact Email: Corresponding author: f.casanova@nanogune.eu; Contact Email: Corresponding author: l.hueso@nanogune.eu; Record automatically processed
Funding organization
'la Caixa' Foundation; Agencia Estatal de Investigación; Narodowa Agencja Wymiany Akademickiej; Euskal Herriko Unibertsitatea