Ionization of oriented targets by intense circularly polarized laser pulses: Imprints of orbital angular nodes in the two-dimensional momentum distribution
- 1. Lundbeck Foundation Theoretical Center for Quantum System Research, Department of Physics and Astronomy, Aarhus University, DK-8000 Aarhus C (Denmark)
Description
We solve the three-dimensional time-dependent Schroedinger equation for a few-cycle circularly polarized femtosecond laser pulse that interacts with an oriented target exemplified by an argon atom, initially in a 3px or 3py state. The photoelectron momentum distributions show distinct signatures of the orbital structure of the initial state as well as the carrier-envelope phase of the applied pulse. Our ab initio results are compared with results obtained using the length-gauge strong-field approximation, which allows for a clear interpretation of the results in terms of classical physics. Furthermore, we show that ionization by a circularly polarized pulse completely maps out the angular nodal structure of the initial state, thus providing a potential tool for studying orbital symmetry in individual systems or during chemical reactions.
Additional details
Identifiers
- DOI
- 10.1103/PhysRevA.81.063418;
- arXiv
- arXiv:1004.1468v1;
Publishing Information
- Journal Title
- Physical Review. A
- Journal Volume
- 81
- Journal Issue
- 6
- Journal Page Range
- p. 063418-063418.7
- ISSN
- 1050-2947
- CODEN
- PLRAAN
INIS
- Country of Publication
- United States
- Country of Input or Organization
- International Atomic Energy Agency (IAEA)
- INIS RN
- 42033909
- Subject category
- S74: ATOMIC AND MOLECULAR PHYSICS;
- Descriptors DEI
- APPROXIMATIONS; ARGON; ATOMS; IONIZATION; LASER RADIATION; PHOTON-ATOM COLLISIONS; POLARIZATION; POTENTIALS; PULSES; SCHROEDINGER EQUATION; TIME DEPENDENCE
- Descriptors DEC
- ATOM COLLISIONS; CALCULATION METHODS; COLLISIONS; DIFFERENTIAL EQUATIONS; ELECTROMAGNETIC RADIATION; ELEMENTS; EQUATIONS; FLUIDS; GASES; NONMETALS; PARTIAL DIFFERENTIAL EQUATIONS; PHOTON COLLISIONS; RADIATIONS; RARE GASES; WAVE EQUATIONS
Optional Information
- Notes
- (c) 2010 The American Physical Society