Published June 2010 | Version v1
Journal article

Ionization of oriented targets by intense circularly polarized laser pulses: Imprints of orbital angular nodes in the two-dimensional momentum distribution

  • 1. Lundbeck Foundation Theoretical Center for Quantum System Research, Department of Physics and Astronomy, Aarhus University, DK-8000 Aarhus C (Denmark)

Description

We solve the three-dimensional time-dependent Schroedinger equation for a few-cycle circularly polarized femtosecond laser pulse that interacts with an oriented target exemplified by an argon atom, initially in a 3px or 3py state. The photoelectron momentum distributions show distinct signatures of the orbital structure of the initial state as well as the carrier-envelope phase of the applied pulse. Our ab initio results are compared with results obtained using the length-gauge strong-field approximation, which allows for a clear interpretation of the results in terms of classical physics. Furthermore, we show that ionization by a circularly polarized pulse completely maps out the angular nodal structure of the initial state, thus providing a potential tool for studying orbital symmetry in individual systems or during chemical reactions.

Additional details

Publishing Information

Journal Title
Physical Review. A
Journal Volume
81
Journal Issue
6
Journal Page Range
p. 063418-063418.7
ISSN
1050-2947
CODEN
PLRAAN

Optional Information

Notes
(c) 2010 The American Physical Society