Pulsed helium droplet beams
Creators
- 1. Department of Chemistry, University of Southern California, Los Angeles, CA 90089 (United States)
- 2. Department of Physics and Astronomy, University of Southern California, Los Angeles, CA 90089 (United States)
Description
Highlights: • Cryogenic pulsed helium droplet beams. • Large helium droplets up to 1011 atoms and 2 μm in diameter. • A factor of ∼1000× higher droplet flux than in continuous beams. • Formation of droplets via the fragmentation of the helium fluid. We report a systematic study of pulsed cryogenic expansion at temperatures ranging from 20 K down to 4.5 K, which enables us to span a large range of helium droplet sizes from ∼105 to ∼1011 He atoms, as obtained via titrations of the droplet beam with helium gas at room temperature. The measured peak flux is a factor of one thousand larger than in a continuous beam. Comparison with continuous nozzle results show similar droplet sizes at low T < 6 K, indicating in both cases the droplets are created via the fragmentation of the fluid.
Availability note (English)
Available from http://dx.doi.org/10.1016/j.cplett.2018.01.035Additional details
Identifiers
- DOI
- 10.1016/j.cplett.2018.01.035;
- PII
- S0009261418300447;
Publishing Information
- Journal Title
- Chemical Physics Letters
- Journal Volume
- 694
- Journal Page Range
- p. 129-134
- ISSN
- 0009-2614
- CODEN
- CHPLBC
INIS
- Country of Publication
- Netherlands
- Country of Input or Organization
- International Atomic Energy Agency (IAEA)
- INIS RN
- 54069373
- Subject category
- S74: ATOMIC AND MOLECULAR PHYSICS;
- Descriptors DEI
- ATOMS; CRYOGENICS; DROPLETS; EXPANSION; HELIUM; NOZZLES; PEAKS; PULSES; TEMPERATURE RANGE 0273-0400 K; TITRATION
- Descriptors DEC
- CHEMICAL ANALYSIS; ELEMENTS; FLUIDS; GASES; NONMETALS; PARTICLES; QUANTITATIVE CHEMICAL ANALYSIS; RARE GASES; TEMPERATURE RANGE; VOLUMETRIC ANALYSIS
Optional Information
- Copyright
- Copyright (c) 2018 Elsevier B.V. All rights reserved.