Published February 2018 | Version v1
Journal article

Pulsed helium droplet beams

  • 1. Department of Chemistry, University of Southern California, Los Angeles, CA 90089 (United States)
  • 2. Department of Physics and Astronomy, University of Southern California, Los Angeles, CA 90089 (United States)

Description

Highlights: • Cryogenic pulsed helium droplet beams. • Large helium droplets up to 1011 atoms and 2 μm in diameter. • A factor of ∼1000× higher droplet flux than in continuous beams. • Formation of droplets via the fragmentation of the helium fluid. We report a systematic study of pulsed cryogenic expansion at temperatures ranging from 20 K down to 4.5 K, which enables us to span a large range of helium droplet sizes from ∼105 to ∼1011 He atoms, as obtained via titrations of the droplet beam with helium gas at room temperature. The measured peak flux is a factor of one thousand larger than in a continuous beam. Comparison with continuous nozzle results show similar droplet sizes at low T < 6 K, indicating in both cases the droplets are created via the fragmentation of the fluid.

Availability note (English)

Available from http://dx.doi.org/10.1016/j.cplett.2018.01.035

Additional details

Identifiers

DOI
10.1016/j.cplett.2018.01.035;
PII
S0009261418300447;

Publishing Information

Journal Title
Chemical Physics Letters
Journal Volume
694
Journal Page Range
p. 129-134
ISSN
0009-2614
CODEN
CHPLBC

INIS

Country of Publication
Netherlands
Country of Input or Organization
International Atomic Energy Agency (IAEA)
INIS RN
54069373
Subject category
S74: ATOMIC AND MOLECULAR PHYSICS;
Descriptors DEI
ATOMS; CRYOGENICS; DROPLETS; EXPANSION; HELIUM; NOZZLES; PEAKS; PULSES; TEMPERATURE RANGE 0273-0400 K; TITRATION
Descriptors DEC
CHEMICAL ANALYSIS; ELEMENTS; FLUIDS; GASES; NONMETALS; PARTICLES; QUANTITATIVE CHEMICAL ANALYSIS; RARE GASES; TEMPERATURE RANGE; VOLUMETRIC ANALYSIS

Optional Information

Copyright
Copyright (c) 2018 Elsevier B.V. All rights reserved.