Harmonic generation by laser-driven classical hydrogen atoms
- 1. Department of Chemistry, Texas A ampersand M University, College Station, Texas 77843-3255 (United States)
- 2. Laboratoire de Chimie Physique, Universite Pierre et Marie Curie, 11 Rue Pierre et Marie Curie, F75231 Paris CEDEX 05 (France)
- 3. Joint Insitute for Laboratory Astrophysics and National Institute of Standards and Technology, University of Colorado, Boulder, Colorado 80309-0440 (United States)
Description
We present the results of our investigations of the dynamics of a classical hydrogen atom submitted to an intense classical radiation field with a relatively low frequency as compared to the characteristic Kepler frequency of the atomic system. We discuss here the harmonic spectra which can be deduced from a Fourier analysis of the time evolution of the strongly driven atomic dipole, associated either with a single trajectory or with ensembles of trajectories evolving from an initial microcanonical distribution. The spectra obtained from ensemble-averaged atomic dipoles qualitatively reproduce the main features of those recently observed in experiments and allow, in particular, discussion of the occurrence of a plateau in the distribution of harmonic intensities as a function of their order. The possible competition between harmonic generation and multiphoton ionization, which both take place in the same laser-intensity range, is also discussed
Additional details
Publishing Information
- Journal Title
- Physical Review. A
- Journal Volume
- 46
- Journal Issue
- 1
- Journal Page Range
- p. 380-390.
- ISSN
- 1050-2947
- CODEN
- PLRAAN
INIS
- Country of Publication
- United States
- Country of Input or Organization
- United States
- INIS RN
- 24021045
- Subject category
- S74: ATOMIC AND MOLECULAR PHYSICS;
- Descriptors DEI
- CLASSICAL MECHANICS; CORRELATIONS; DIPOLES; HARMONIC GENERATION; HYDROGEN; LASERS; MULTI-PHOTON PROCESSES; PHOTOIONIZATION; PHOTON-ATOM COLLISIONS; RESONANCE; SPECTRAL SHIFT
- Descriptors DEC
- AMPLIFIERS; ATOM COLLISIONS; COLLISIONS; ELEMENTS; EQUIPMENT; IONIZATION; MECHANICS; MULTIPOLES; NONMETALS; PHOTON COLLISIONS