Published May 23, 2007 | Version v1
Journal article

Critical fluctuations and breakdown of the Stokes-Einstein relation in the mode-coupling theory of glasses

  • 1. Service de Physique Theorique Centre d'Etudes de Saclay, Orme des Merisiers, 91191 Gif-sur-Yvette Cedex (France)
  • 2. Service de Physique de l'Etat Condense, Orme des Merisiers, CEA Saclay, 91191 Gif sur Yvette Cedex (France)

Description

We argue that the critical dynamical fluctuations predicted by the mode-coupling theory (MCT) of glasses provide a natural mechanism to explain the breakdown of the Stokes-Einstein relation. This breakdown, observed numerically and experimentally in a region where MCT should hold, is one of the major difficulties of the theory, for which we propose a natural resolution based on the recent interpretation of the MCT transition as a bona fide critical point with a diverging length scale. We also show that the upper critical dimension of MCT for liquids is dc = 8

Additional details

Identifiers

DOI
10.1088/0953-8984/19/20/205101;
PII
S0953-8984(07)34501-3;

Publishing Information

Journal Title
Journal of Physics. Condensed Matter
Journal Volume
19
Journal Issue
20
Journal Page Range
p. 205101
ISSN
0953-8984
CODEN
JCOMEL

INIS

Country of Publication
United Kingdom
Country of Input or Organization
International Atomic Energy Agency (IAEA)
INIS RN
38077859
Subject category
S75: CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY;
Descriptors DEI
COUPLING; FLUCTUATIONS; GLASS; LENGTH; LIQUIDS; PHASE STABILITY; PHASE STUDIES; PHASE TRANSFORMATIONS
Descriptors DEC
DIMENSIONS; FLUIDS; STABILITY; VARIATIONS