Published May 23, 2007
| Version v1
Journal article
Critical fluctuations and breakdown of the Stokes-Einstein relation in the mode-coupling theory of glasses
Creators
- 1. Service de Physique Theorique Centre d'Etudes de Saclay, Orme des Merisiers, 91191 Gif-sur-Yvette Cedex (France)
- 2. Service de Physique de l'Etat Condense, Orme des Merisiers, CEA Saclay, 91191 Gif sur Yvette Cedex (France)
Description
We argue that the critical dynamical fluctuations predicted by the mode-coupling theory (MCT) of glasses provide a natural mechanism to explain the breakdown of the Stokes-Einstein relation. This breakdown, observed numerically and experimentally in a region where MCT should hold, is one of the major difficulties of the theory, for which we propose a natural resolution based on the recent interpretation of the MCT transition as a bona fide critical point with a diverging length scale. We also show that the upper critical dimension of MCT for liquids is dc = 8
Additional details
Identifiers
- DOI
- 10.1088/0953-8984/19/20/205101;
- PII
- S0953-8984(07)34501-3;
Publishing Information
- Journal Title
- Journal of Physics. Condensed Matter
- Journal Volume
- 19
- Journal Issue
- 20
- Journal Page Range
- p. 205101
- ISSN
- 0953-8984
- CODEN
- JCOMEL
INIS
- Country of Publication
- United Kingdom
- Country of Input or Organization
- International Atomic Energy Agency (IAEA)
- INIS RN
- 38077859
- Subject category
- S75: CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY;
- Descriptors DEI
- COUPLING; FLUCTUATIONS; GLASS; LENGTH; LIQUIDS; PHASE STABILITY; PHASE STUDIES; PHASE TRANSFORMATIONS
- Descriptors DEC
- DIMENSIONS; FLUIDS; STABILITY; VARIATIONS