Published September 1, 2007 | Version v1
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Entrance-channel effects in odd-Z tranactinide compound nucleus reactions

Description

Swiatecki, Siwek-Wilczynska, and Wilczynski's 'Fusion By Diffusion' description [1] of transactinide (TAN) compound nucleus (CN) formation utilizes a three-step model. The first step is the 'sticking', or capture, which can be calculated relatively accurately. The second step is the probability for the formation of a CN by 'diffusion' analogous to that of Brownian motion. Lastly, there exists the probability of the CN 'surviving' deexcitation by neutron emission, which competes with fission and other de-excitation modes. This model predicts and reproduces cross sections typically within a factor of two. Producing the same CN with different projectile-target pairs is a very sensitive way to test entrance channel effects on heavy element production cross sections. If the same CN is produced at or near the same excitation energy the survival portion of the theory is nearly identical for the two reactions. This method can be used as a critical test of the novel 'diffusion' portion of the model. The reactions producing odd-Z TAN CN such as Db, Bh, Mt, and Rg (Z = 105, 107, 109, and 111, respectively) were first studied using even-Z projectiles on 209Bi targets (as opposed to odd-Z projectiles on 208Pb targets) because lower effective fissility [2] was expected to lead to larger cross sections. Many odd-Z projectile reactions producing odd-Z CN had not been studied in-depth until very recently. We have completed studies of these reaction pairs with the 88-Inch Cyclotron and the Berkeley Gas-Filled Separator (BGS) at the Lawrence Berkeley National Laboratory (LBNL), see Figure 1. Cross section ratios for several pairs of reactions will be presented and compared with theory

Availability note (English)

Available from INIS in electronic form; Also available from OSTI as DE00939486; PURL: https://www.osti.gov/servlets/purl/939486-ojgbrl/

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Additional details

Publishing Information

Imprint Pagination
1 p.
Report number
LBNL--227E-Ext-Abs

Conference

Title
3. International Conference on the Chemistry and Physics of the Transactinide Elements
Dates
23-28 Sep 2007
Place
Davos (Switzerland)

INIS

Country of Publication
United States
Country of Input or Organization
United States
INIS RN
40007627
Subject category
S73: NUCLEAR PHYSICS AND RADIATION PHYSICS;
Resource subtype / Literary indicator
Conference
Descriptors DEI
CHEMISTRY; COMPOUND-NUCLEUS REACTIONS; CROSS SECTIONS; CYCLOTRONS; DE-EXCITATION; DIFFUSION; EXCITATION; FISSION; NEUTRON EMISSION; PROBABILITY; TARGETS; TRANSACTINIDE ELEMENTS
Descriptors DEC
ACCELERATORS; CYCLIC ACCELERATORS; ELEMENTS; EMISSION; ENERGY-LEVEL TRANSITIONS; NUCLEAR REACTIONS; TRANSPLUTONIUM ELEMENTS; TRANSURANIUM ELEMENTS

Optional Information

Contract/Grant/Project number
AC02-05CH11231
Funding organization
Nuclear Science Division (United States)