The GSF anticoincidence-shielded Ge(Li) gamma-ray spectrometer and its application to the analysis of environmental samples

A high-efficiency gamma-ray spectrometer has been designed and built to provide simultaneous anticoincidence and coincidence spectrometry of low-level environmental samples. The spectrometer consists of a large-volume Ge(Li) detector as the main detector and a well-type NaI(Tl) guard detector. The Ge(Li) detector is a closed-end coaxial detector housed in a crystal of the vertical dip-stick type. Its relative photopeak efficiency is 27.5%. The guard counter is a 23-cm-dia. by 23-cm-long NaI(Tl) crystal with a 7.8-cm-dia. by 18-cm-deep centre well. The passive shield consists of a 10-cm lead shield with copper and cadmium lining. The electronics is designed to operate independently and simultaneously in the anticoincidence mode as well as in the coincidence or in the normal passive shield mode. When operating in the anticoincidence mode the Compton edge of 137Cs is reduced by a factor of 7.7 to provide a peak-to-Compton edge ratio of 480:1. Bulk samples up to about 300 cm3 can be measured on the top of the detector end cap inside the well of the NaI(Tl) crystal. The lower limit of detection (1000 min counting time, 95% confidence level) for 137Cs is 1.6 pCi in a 3.8-cm-dia. by 3.5-cm-high sample geometry. The design of the spectrometer, its properties and the application to investigations on the migration of radionuclides in the soil, the analysis of radioactive emissions of coal-fired power plants and to fallout studies are described. (author)