In-line measurement of total and isotopic plutonium concentrations by gamma-ray spectrometry

Preliminary experiments studying the feasibility of gamma-ray spectrometry for in-line measurements of plutonium in solutions are described. The isotopic content of the plutonium was measured by direct counting and the total plutonium content by a differential attenuation technique. Two separate experiments on different solutions were performed with each technique. Our results show that both isotopic and total measurements can be made with precisions around 0.25 to 0.5 percent