Published May 2, 1994 | Version v1
Journal article

Observed frustration in confined block copolymers

  • 1. IBM Research Division, Almaden Research Center, 650 Harry Road, San Jose, California 95120-6099 (United States)
  • 2. Department of Materials Science and Engineering, Massachusetts Institute of Technology, Cambridge, Massachusetts 02139 (United States)
  • 3. Reactor and Radiation Division, National Institute for Standards Technology, Gaithersburg, Maryland 60439 (United States)

Description

Symmetric diblock copolymers confined between two solid surfaces were studied by neutron reflectivity. A multilayered morphology with an integral number of layers oriented parallel to the solid interfaces was found in all cases. The period of the confined multilayers deviated from the bulk period in a cyclic manner as a function of the confined film thickness. A first-order transition occurred between the expanded and contracted states of the copolymer chains. The data suggest that the deviation of the period from the bulk value decreases with increasing separation distance

Additional details

Publishing Information

Journal Title
Physical Review Letters
Journal Volume
72
Journal Issue
18
Journal Page Range
p. 2899-2902.
ISSN
0031-9007
CODEN
PRLTAO