Electrophoretic deposition of high quality transparent conductive graphene films on insulating glass substrates

Graphene is a promising material for transparent conductive films (TCFs) because of its high electrical conductivity and excellent optical transparency over a wide spectral range. We have previously reported on an inexpensive means of producing graphene-based TCFs using chemically derived graphene flakes. However, the deposition of chemically derived graphene can yield poor stacking of graphene flakes, which degrades the electrical conductivity of the resulting films. Here, we describe an alternative approach for producing large areas of TCFs based on electrophoretic deposition of graphene onto glass substrates using charged graphene oxide flakes. This method enabled the deposition of highly stacked graphene films onto insulating glass substrates with potential for TCFs.