Published 1998 | Version v1
Journal article

Problems of unusual hydrogen bonds between proton donors and hydrides of transition metals and boron

  • 1. Inst. Ehlementoorganicheskikh Soedinenij im. A.N. Nesmeyanova RAN, Moscow (Russian Federation)

Description

Results of experimental and theoretical studies on intermolecular hydrogen bonds with hydride atom as a proton acceptor site MH...HX (M = W, Re, Ru) and BH...HX were analyzed. Spectral (IR and NMR) criteria of such hydrogen bonds formation were found. Spectral, structural, and thermodynamic characteristics of these unusual hydrogen bonds are governed by regularities found for classical hydrogen bonds. The participation of MH...HX bonds in proton transfer with the formation of cationic nonclassical hydrides as well as formation of hydrogen bonds [M(η2-H2)]+ ... A- in low polar media was demonstrated. Problems arising in this new area are discussed

Additional details

Additional titles

Original title (Russian)
Проблемс необычных водородных связей доноров протона с гидридами переходных металлов и бора

Publishing Information

Journal Title
Izvestiya Akademii Nauk. Rossijskaya Akademiya Nauk. Seriya Khimicheskaya
Journal Issue
no.5
Journal Page Range
p. 846-851
ISSN
0002-3353
CODEN
IASKEA

Optional Information

Notes
30 refs.; 2 figs.