Published December 1987 | Version v1
Journal article

Solvent extraction of thorium from mixed organic-aqueous nitric acid media by tri-n-octylphosphine oxide

  • 1. University of Garyounis, Benghazi (Libya). Dept. of Chemistry and Physics

Description

The extraction equilibria of Th in tri-n-octylphosphine oxide (TOPO)-HNO3-H2O systems were investigated in the absence and presence of water-miscible alcohols and acetone. The influence of TOPO concentration in an inert diluent (toluene) and the concentration of nitric acid and the water-miscible additives were systematically examined. The slopes of the log-log plots of DTh vs. the TOPO concentration (up to 0.02M) are found to be close to 3 over a wide range of polar phase compositions leading to a coordination number of 11 for Th. The results show that at TOPO concentrations above about 2.5x10-3M (about 1 %) in toluene, polymerization of the solvent occurs. (author) 23 refs

Additional details

Publishing Information

Journal Title
J. Radioanal. Nucl. Chem.
Journal Volume
116
Journal Issue
2
Series
J. Radioanal. Nucl. Chem. ;Articles.
Journal Page Range
271-284
ISSN
0236-5731
CODEN
JRNCD