Published 2016 | Version v1
Journal article

Recent progress of radiation physicochemical process. Second part

  • 1. Japan Atomic Energy Agency, Tokai, Ibaraki (Japan)
  • 2. National Institutes for Quantum and Radiological Science and Technology, Chiba (Japan)

Description

The thermalization length and spatial probability distribution of electrons in liquid water were simulated for initial electron energies ranging from 0.1 eV to 1 x 105 eV using a dynamic Monte Carlo code. The results showed that electrons were decelerated for thermalization over a longer time period than was previously predicted. This long thermalization time significantly contributed to the series of processes from initial ionization to hydration. We further studied the particular deceleration process of electrons at an incident energy of 1 eV, focusing on the temporal evolution of total track length, mean traveling distance, and energy distributions of decelerating electrons. The initial prehydration time and thermalization periods were estimated to be approximately 50 fs and 220 fs, respectively, indicating that the initial prehydration began before or contemporaneously with the thermal equilibrium. (author)

Additional details

Additional titles

Original title (Japanese)
放射線物理化学過程に関する最近の進展(中編)

Publishing Information

Journal Title
Hoshasen Kagaku (Online)
Journal Issue
no.102
Series
雑誌名:放射線化学
Journal Page Range
p. 49-56
ISSN
2188-0115

Optional Information

Notes
26 refs., 8 figs.