Published January 1992 | Version v1
Journal article

Regularities of redox reactions in mixtures of carbides and oxides of 4A-5A group metals

Description

Methods of thermodynamic, kinetic and X-ray phase, thermal and mass-spectrometric analysis are used to study the main regularities of phase formation in MC1-x+MmOn (M=Ti, Zr, V, Nb) reaction mixtures in the temperature range up to 1870 K. It is stated that interaction in the given systems is characterized by consecutive reduction of higher oxide (excluding ZrO2) up to M2O3 (M=Ti, V) or MO2 (M=Nb), subsequent formation of oxycarbide phases by MC1-x+M2O3(MO2) → MOzCy + CO chemical reaction, dissolution of the formed oxycarbide in initial isostructural carbide. In M5C1-x + Mm5On mixtures the process is completed by formation of M2C(O) hexagonal oxycarbide or a metal

Additional details

Additional titles

Original title (Russian)
Закономерности окислительно-восстановительных реакций в смесях карбидов и оксидов металлов 4A-5A групп

Publishing Information

Journal Title
Zhurnal Neorganicheskoj Khimii
Journal Volume
37
Journal Issue
1
Journal Page Range
p. 3-10.
ISSN
0044-457X
CODEN
ZNOKAQ