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AbstractAbstract
[en] Using data for the discharge of effluents to the Irish Sea, from the nuclear fuel reprocessing plant at Windscale, the probable sedimentary deposition of 241 Am and 241Pu over the past 20 yr is estimated and the consequent additional ingrowth of 241Am, due to decay of 241Pu, is calculated. The latter is now approximately 600 Ci yr-1, rising towards a steady state approximately 1,300 Ci yr-1 if present rates of discharge of 241Pu are maintained. The present sedimentary reservoir of 241Am is approximately 18,000 Ci, of which about 4,800 have resulted from 241Pu decay in situ. Measurements of the 241Pu/Pu-α isotope ratio in coastal sediments confirms the estimates of 241Pu deposition. Outside the Irish Sea, in the dispersal plume into Scottish waters, it is concluded that the observed 241Am concentration can be accounted for largely by ingrowth from the 241Pu transported in the water mass. (U.K.)
Primary Subject
Record Type
Journal Article
Literature Type
Numerical Data
Journal
Nature (London); ISSN 0028-0836;
; v. 292(5818); p. 43-45

Country of publication
ACTINIDE NUCLEI, ALPHA DECAY RADIOISOTOPES, AMERICIUM ISOTOPES, ATLANTIC OCEAN, BETA DECAY RADIOISOTOPES, BETA-MINUS DECAY RADIOISOTOPES, DATA, DECAY, EVEN-ODD NUCLEI, HEAVY NUCLEI, INFORMATION, ISOTOPES, MANAGEMENT, NUCLEAR DECAY, NUCLEAR FACILITIES, NUCLEI, NUMERICAL DATA, ODD-EVEN NUCLEI, PLUTONIUM ISOTOPES, RADIOACTIVE MATERIALS, RADIOACTIVE WASTES, RADIOISOTOPES, SEAS, SURFACE WATERS, WASTE DISPOSAL, WASTE MANAGEMENT, WASTES, YEARS LIVING RADIOISOTOPES
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