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Mishima, J.; Lindsey, C.G.
Pacific Northwest Lab., Richland, WA (USA)1983
Pacific Northwest Lab., Richland, WA (USA)1983
AbstractAbstract
[en] Pacific Northwest Laboratory (PNL), operated for the Department of Energy by the Battelle Memorial Institute, is conducting a study for the Nuclear Regulatory Commission on the feasibility of altering current plutonium shipping forms to reduce or eliminate the airborne dispersibility of PuO2 which might occur during a shipping accident. Plutonium used for fuel fabrication is currently shipped as a PuO2 powder with a significant fraction in the respirable size range. If the high-strength container is breached due to stresses imposed during a transportation accident, the PuO2 powder could be subject to airborne dispersion. The available information indicated that a potential accident involving fire accompanied by crush/impact forces would lead to failure of current surface shipping containers (no assumptions were made on the possibility of such a severe accident). Criteria were defined for an alternate shipping form to mitigate the effects of such an accident. Candidate techniques and materials were evaluated as alternate shipping forms by a task team consisting of personnel from PNL and Rockwell Hanford Operations (RHO). At this time, the most promising candidate for an alternate plutonium shipping form appears to be pressing PuO2 into unsintered (green) pellets. These green pellets satisfy the criteria for a less dispersible form without requiring significant process changes. Discussions of all candidates considered are contained in a series of appendices. Recommendations for further investigations of the applicability of green pellets as an alternate shipping form are given, including the need for a cost-benefit study
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Jun 1983; 164 p; PNL--4507; Available from NTIS, PC A08/MF A01 - GPO $6.00 as DE83014373
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