Filters
Results 1 - 1 of 1
Results 1 - 1 of 1.
Search took: 0.012 seconds
Curtis, D.B.; Benjamin, T.M.; Gancarz, A.J.
Technology of high-level nuclear waste disposal. Advances in the science and engineering of the management of high-level nuclear wastes. Volume 11981
Technology of high-level nuclear waste disposal. Advances in the science and engineering of the management of high-level nuclear wastes. Volume 11981
AbstractAbstract
[en] The 2-billion-year-old fossil reactors at Oklo are ancient natural nuclear waste sites. Isotope dilution mass spectrometric analyses of the fission products in the reactor core uraninite and the peripheral pelitic sandstone provide data for calculating the reactor operating parameters, the quantities of fissiogenic isotopes produced, the fraction of these isotopes retained in the cores, and the location in the peripheral rocks of the fissiogenic fraction lost from the cores. For a duration of criticality of 3 x 105 yrs, the thermal plus resonance neutron fluence ranged between 1020 and 1021 neutrons/cm2. The fraction of technetium (60 to 85%), ruthenium (75 to 90%), and neodymium (85 to 100%) retained is negatively correlated with fluence. The lost fission products are contained within a few tens of meters of their source, the reactor cores. The systematics of the decay of 99Tc (t12/ = 2.13 x 105 yr) to 99Ru limits the period of fissiogenic element migration to approximately 1 million yr at a time 2 billion yr ago. Thermodynamic calculations of the temperature-dependent solubilities indicate that the loss of fissiogenic elements is diffusion controlled, whereas retention in the surrounding rocks is a result of temperature-dependent deposition from an aqueous solution. These results concerning the geochemistry of technetium, ruthenium, and neodymium at a natural waste site support the concept of geologic burial of man-made radioactive wastes
Primary Subject
Secondary Subject
Source
Hofmann, P.L.; Breslin, J.J. (eds.); Department of Energy, Oak Ridge, TN (USA). Technical Information Center; p. 255-283; 1981; p. 255-283; Available from NTIS $18.00 as DE82009594
Record Type
Report
Report Number
Country of publication
Reference NumberReference Number
INIS VolumeINIS Volume
INIS IssueINIS Issue