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AbstractAbstract
[en] The steady state release of active noble gas and iodine from defective fuel elements is described in terms of either a kinetic or a diffusion model. Both models assume a diffusional release in the fuel. However, transport of fission products in the fuel-to-sheath gap is represented either by a first-order rate process or by a diffusion process, and is characterized with an escape-rate constant or a diffusion coefficient, respectively. The kinetic model predicts a release dependence on the decay constant of λ/sup -1/2/ to λ/sup -3/2/, whereas the diffusion model predicts a release dependence of λ/sup -1/. Observed release data from in-pile loop experiments, for a wide range of defect states, confirm these predicted dependencies, A fit of the model to the measured data yields estimates of the empirical diffusion coefficient in the fuel matrix, and the escape-rate constant or the diffusion coefficient in the fuel-to-sheath gap. Evaluation of the fitted parameters enables the various rate-controlling processes to be deduced as a function of the defect size
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Source
Hastings, I.J; p. 95-106; ISBN 0-86531-603-1;
; 1986; p. 95-106; American Ceramic Society; Columbus, OH (USA); American Ceramic Society annual meeting; Cincinnati, OH (USA); 5-9 May 1985

Record Type
Book
Literature Type
Conference
Country of publication
DATA PROCESSING, DECAY, DEFECTS, DIFFUSION, FISSION PRODUCT RELEASE, FUEL CANS, FUEL ELEMENTS, FUEL-CLADDING INTERACTIONS, GASEOUS WASTES, IODINE ISOTOPES, KINETIC EQUATIONS, MATHEMATICAL MODELS, RADIOACTIVE WASTES, RARE GASES, RESEARCH PROGRAMS, SIZE, STEADY-STATE CONDITIONS, URANIUM DIOXIDE, ZIRCALOY
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