Filters
Results 1 - 1 of 1
Results 1 - 1 of 1.
Search took: 0.016 seconds
Apted, M.J.; Engel, D.W.
Pacific Northwest Lab., Richland, WA (USA)1988
Pacific Northwest Lab., Richland, WA (USA)1988
AbstractAbstract
[en] The Analytical Repository Source-Term (AREST) code has been developed for source-term evaluation of spent fuel as a final waste form in geologic repositories. AREST contains a set of analytical equations for the time-dependent diffusional mass transport of both solubility-limited and inventory-limited radionuclides from a spent fuel in a failed container surrounded by a shell of packing or other porous material imbedded in a porous host rock. Three factors that affect release performance are congruent dissolution of the UO2 matrix: chemical instability of the UO2 matrix, with precipitation of a more stable uranium phase within the waste package: and the attenuation of release rate by distribution of containment failures with time. For congruent matrix dissolution, the release rates of included nuclides are proportional to the product of solubility-limited release of uranium and the fractional abundance of the nuclide. For certain conditions, congruent release rates are calculated to be up to 10 orders of magnitude lower than release rates assuming individual solubility-limits. Precipitation of a more stable, lower solubility uranium phase within the waste package is shown to increase release rates from the UO2 matrix compared to the non-precipitation case, in agreement with previous calculations. During the first 300 to 1000 years after repository closure, the distribution of containment failures with time will act to attenuate the peak average release rates of soluble, long-lived nuclides, such as iodine-129, to values smaller than release rates below regulatory limits. 27 refs., 5 figs
Primary Subject
Secondary Subject
Source
Mar 1988; 11 p; Fall meeting of the Materials Research Society; Boston, MA (USA); 30 Nov - 5 Dec 1987; CONF-871124--95; Available from NTIS, PC A03/MF A01 as DE88008177
Record Type
Report
Literature Type
Conference
Report Number
Country of publication
Reference NumberReference Number
INIS VolumeINIS Volume
INIS IssueINIS Issue