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Haigh, D.G.; Hooker, P.J.
Department of the Environment, London (UK)1988
Department of the Environment, London (UK)1988
AbstractAbstract
[en] A number of radionuclide batch sorption tests have been carried out on core material from boreholes on the BNFL Drigg site, Cumbria, as part of an intercomparison exercise with BNFL, Sellafield. This report describes the nature of the materials used, the method and the results of the BGS side of the interlaboratory exercise. Another report will describe the intercomparison. These experiments formed part of a wider programme of laboratory tests by BGS to ascertain the sorption properties of the Drigg sands and silts as an information base for designing artificial in-situ radionuclide migration experiments on site at Drigg. Three radionuclides were used, 85Sr, 137Cs, and 227Th. Interestingly, although sorption of strontium was about 15 times less than for thorium, the pattern of sorption as a function of borehole depth i.e. mineralogical composition, was very similar. Sorption of 137Cs was found to be non-linear, depending strongly on caesium concentration in the groundwater. Isotherm fits were used to determine the energy of sorption in the ion exchange process, the mechanism responsible for uptake. There is a need for a standard batch sorption method to be in common use. (author)
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Apr 1988; 43 p; CONTRACT PECD-7/9/306; WE/88/16
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Report
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ACTINIDE NUCLEI, ALPHA DECAY RADIOISOTOPES, BETA DECAY RADIOISOTOPES, BETA-MINUS DECAY RADIOISOTOPES, CESIUM ISOTOPES, DAYS LIVING RADIOISOTOPES, ELECTRON CAPTURE RADIOISOTOPES, ENVIRONMENTAL TRANSPORT, EVEN-ODD NUCLEI, HEAVY NUCLEI, HOURS LIVING RADIOISOTOPES, INTERMEDIATE MASS NUCLEI, ISOMERIC TRANSITION ISOTOPES, ISOTOPES, MASS TRANSFER, NUCLEI, ODD-EVEN NUCLEI, RADIOISOTOPES, STRONTIUM ISOTOPES, THORIUM ISOTOPES, YEARS LIVING RADIOISOTOPES
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