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Wilson, C.N.; Bruton, C.J.
Pacific Northwest Lab., Richland, WA (USA)1989
Pacific Northwest Lab., Richland, WA (USA)1989
AbstractAbstract
[en] Nuclide concentrations measured in laboratory tests with PWR spent fuel specimens in Nevada Test Site J-13 well water are compared to equilibrium concentrations calculated using the EQ3/6 geochemical modeling code. Actinide concentrations in the laboratory tests reach steady-state values lower than those required to meet Nuclear Regulatory Commission (NRC) release limits. Differences between measured and calculated actinide concentrations are discussed in terms of the effects of temperature (25 degree C to 90 degree C), sample filtration, oxygen fugacity, secondary phase precipitation, and the thermodynamic data in use. The concentrations of fission product radionuclides in the laboratory tests tend to increase continuously with time, in contrast to the behavior of the actinides. 11 refs., 5 figs., 4 tabs
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Jul 1989; 19 p; 91. annual meeting of the American Ceramic Society; Indianapolis, IN (USA); 23-27 Apr 1989; CONF-890421--11; CONTRACT AC06-76RL01830; W-7405-ENG-48; Available from NTIS, PC A03/MF A01 as DE89017242; OSTI; INIS; US Govt. Printing Office Dep
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