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Wang, L.M.; Ewing, R.C.; Eby, R.K.
Pacific Northwest Lab., Richland, WA (United States). Funding organisation: USDOE, Washington, DC (United States); National Aeronautics and Space Administration, Washington, DC (United States)1992
Pacific Northwest Lab., Richland, WA (United States). Funding organisation: USDOE, Washington, DC (United States); National Aeronautics and Space Administration, Washington, DC (United States)1992
AbstractAbstract
[en] The temperature dependence of amorphization dose for zircon under 1.5 MeV Kr ion irradiation has been investigated using the ANL HVEM-Tandem Facility. Three regimes were observed in the amorphization dose-temperature curve. In the first regime (15 to 300 K), the critical amorphization dose increased from 3.06 to 4.5 ions/nm2. In the second regime (300 to 473 K), there is little change in the amorphizationdose. In the third regime (> 473 K), the amorphization dose increased exponentially to 8.3 ions/nm2 at 913 K. This temperature dependence of amorphization dose can be described by two processes with different activation energies (0.018 and 0.31 eV respectively) which are attributed to close pair recombination in the cascades at low temperatures and radiation-enhanced epitaxial recrystallization at higher temperatures. The upper temperature limit for amorphization of zircon is estimated to be 1100 K. The ion-mass dependence of the amorphization dose (in dpa) has also been discussed in terms of the energy to recoils based on data obtained from He, Ne, Ar, Kr, Xe irradiations and a 238Pu-doped sample
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Dec 1992; 7 p; 16. International Symposium on the Scientific Basis for Nuclear Waste Management as Part of the Fall Meeting of the Materials Research Society (MRS); Boston, MA (United States); 30 Nov - 4 Dec 1992; CONF-921101--95; CONTRACT AC06-76RL01830; FG04-84ER45099; OSTI as DE93007881; NTIS; INIS; US Govt. Printing Office Dep
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