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Hopper, C.M.; Wright, R.Q.; Elam, K.R.; Forsberg, C.W.
Oak Ridge National Lab., TN (United States). Funding organisation: USDOE Office of Fissile Materials Disposition, Washington, DC (United States)1997
Oak Ridge National Lab., TN (United States). Funding organisation: USDOE Office of Fissile Materials Disposition, Washington, DC (United States)1997
AbstractAbstract
[en] The disposal of excess 233U as waste is being considered. Because 233U is a fissile material, a key requirement for processing 233U to a final waste form and disposing of it is the avoidance of nuclear criticality. For many processing and disposal options, isotopic dilution is the most feasible and preferred option to avoid nuclear criticality. Isotopic dilution is dilution of fissile 233U with nonfissile 238U. The use of isotopic dilution removes any need to control nuclear criticality in process or disposal facilities through geometry or chemical composition. Isotopic dilution allows the use of existing waste management facilities that are not designed for significant quantities of fissile materials to be used for processing and disposing of 233U. The amount of isotopic dilution required to reduce criticality concerns to reasonable levels was determined in this study to be approximately 0.53 wt % 233U. The numerical calculations used to define this limit consisted of a homogeneous system of silicon dioxide (SiO2), water (H2O), 233U and depleted uranium (DU) in which the ratio of each component was varied to learn the conditions of maximum nuclear reactivity. About 188 parts of DU (0.2 wt % 235U) are required to dilute 1 part of 233U to this limit in a water-moderated system with no SiO2 present. Thus for the U.S. inventory of 233U, several hundred metric tons of DU would be required for isotopic dilution
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1997; 6 p; American Nuclear Society (ANS) topical meeting on criticality challenges in the next decade; Chelan, WA (United States); 7-10 Sep 1997; CONTRACT AC05-96OR22464; Also available from OSTI as DE97006434; NTIS; US Govt. Printing Office Dep
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Report
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Conference
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ACTINIDE NUCLEI, ACTINIDES, ALPHA DECAY RADIOISOTOPES, ELEMENTS, EVEN-ODD NUCLEI, FISSIONABLE MATERIALS, HEAVY ION DECAY RADIOISOTOPES, HEAVY NUCLEI, ISOTOPE APPLICATIONS, ISOTOPES, MANAGEMENT, MATERIALS, METALS, NEON 24 DECAY RADIOISOTOPES, NUCLEI, RADIOISOTOPES, SPONTANEOUS FISSION RADIOISOTOPES, TRACER TECHNIQUES, URANIUM, URANIUM ISOTOPES, WASTE DISPOSAL, WASTE MANAGEMENT, YEARS LIVING RADIOISOTOPES
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