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AbstractAbstract
[en] The magnetic properties of CePtAl with orthorhombic TiNiSi-type chemical structure were investigated. Single-crystal experiments of electrical resistivity, specific heat and magnetic susceptibility reveal the existence of three magnetic phase transitions at T1 = 5.9 K (second order), T2 = 4.3 K (first order) and T3 = 2.2 K (first order). Powder neutron diffraction measurements detected complex magnetic structures consisting of two coexisting, partly incommensurate magnetic propagation vectors: k1=0 and k3=(0, 0.463(8), 0) for T2≤T≤T1; and k1=0 and k2 = (0, 1/2, 0) for T≤T2. The predominantly ferromagnetic k1 component and the antiferromagnetic k2 component of the magnetic low-temperature structure of CePtAl were refined at 1.5 K. Magnetism in CePtAl is dominated by a ferromagnetic component (1.35(4) μB at 1.5 K) oriented parallel to the magnetically easy a axis. The complexity of magnetic structures in CePtAl appears to be caused by competing anisotropic magnetic exchange interactions in a network, where Ce-Ce nearest neighbours (3.56 AA) form chains parallel to the b axis and Ce-Ce second-nearest neighbours (3.77 AA) form chains along the a axis. (author)
Source
Available online at the Web site for the Journal of Physics. Condensed Matter (ISSN 1361-648X) http://www.iop.org/; Country of input: Portugal
Record Type
Journal Article
Literature Type
Numerical Data
Journal
Journal of Physics. Condensed Matter; ISSN 0953-8984;
; v. 7(8); p. 1663-1678

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