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AbstractAbstract
[en] The crystal-field transitions in the paramagnetic state of PrCu2 were studied by means of inelastic neutron scattering between 1.8 and 10 K in an energy transfer range 0.5-2.5 meV. We observed excitations from the singlet ground state to two singlet excited states. They were assigned as a Jx-polarized and a Jy-polarized transition. The Jx transition has acoustic and optical branches. While the Jy transition is very weakly dependent on the wavenumber, the Jx transitions are strongly dispersive, indicating an anisotropic RKKY interaction between the 4f electrons. A substantial softening of the exciton energy was observed in the optical branch of the Jx transition as a sharp minimum at the wavevector Qm=0.24a*+0.68c*, which is the modulation vector of the magnetic order below TN = 54 mK. The manner of softening above 1.8 K is discussed in terms of the mean-field theory. (author)
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Available online at the Web site for the Journal of Physics. Condensed Matter (ISSN 1361-648X) http://www.iop.org/; Country of input: Uzbekistan
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Journal Article
Journal
Journal of Physics. Condensed Matter; ISSN 0953-8984;
; v. 7(21); p. 4051-4059

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