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Gaizauskas, E.; Feller, K.-H., E-mail: feller@fh-jena.de2003
AbstractAbstract
[en] We have studied the effects of induced off-diagonal disorder on pump-probe spectra in J-aggregates. Changes of the disorder, i.e. randomness in excite energy of site molecules and inter-molecular coupling within a meso-aggregates, is considered by introducing different random Hamiltonian matrices for two ensembles of aggregates. The theory allows to interpret the intensity-dependent spectra on the J-aggregates as contributed from the combined action of exciton-exciton annihilation and subsequent dynamic disordering processes. The possibility of the transient stage of aggregate ensembles exhibiting lasing due to the excess off-diagonal disorder is demonstrated
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2002 international conference on luminescence and optical spectroscopy of condensed matter; Budapest (Hungary); 24-29 Aug 2002; S0022231302005446; Copyright (c) 2002 Elsevier Science B.V., Amsterdam, The Netherlands, All rights reserved.; Country of input: International Atomic Energy Agency (IAEA)
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