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AbstractAbstract
[en] Our first countrywide study carried out in 1991-1993 determined both geographical and depth distributions of the deposited 134Cs and 137Cs in the Estonian soil. According to the results of this study and an independent air-borne scanning, radiocaesium originating from the 1986 Chernobyl accident with the mean deposition of 2 kBq m-2 was extremely unevenly distributed over the country . The mapped distribution is presented in Fig. 1. Our estimates demonstrated that about 2/3 of the total 137Cs inventory in Estonia was deposited in Ida-Virumaa County, NE Estonia, where the maximum depositions reached 40 kBq m-2. The region was revisited for soil sampling in 1998-2001. Undisturbed soil profiles down to a depth of ∼ 20 cm were collected and the 2-3 cm sample core slices analyzed using a low-background HPGe gamma spectrometer (42% efficiency and 1.7 keV resolution). As in the previous study, both total depositions and depth distributions of the deposited 134Cs (where possible) and 137Cs activity concentrations were determined. Depth distributions of the deposited activity showed considerable site-specific variations. In addition, it appeared that in comparison with our previous study, clear features of time-dependent migration to deeper soil layers were evident. The preliminary modeling has demonstrated that a lognormal distribution with varying parameters fits satisfactorily the determined depth-distributions of the Chernobyl radiocaesium activity concentration. An attempt was made to apply a single model to describe the observed time-dependent depth-distribution pattern over the time period of 1986-2001. We started from the multi-compartmental migration model for undisturbed soil (here Model RP72), presented in Fig. 2. This model has been elaborated basing on experimental migration results for Pu for a time period up to 30 y. For our application, the model is modified to account for the radioactive decay of 137Cs. The results of modeling using the original transfer parameters are given in Fig. 3 (a)
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Source
D'Alberti, F.; Osimani, C. (eds.); Associazione Italiana di Radioprotezione, (Italy); International Radiation Protection Association, (United States); [1 CD-ROM]; ISBN 88-88648-09-7;
; 2002; [3 p.]; European IRPA Congress 2002; Florence (Italy); 8-11 Oct 2002; Also available from http://www.airp-asso.it/docs/cd_airp_irpa/irpa2002.pdf

Record Type
Miscellaneous
Literature Type
Conference
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BETA DECAY RADIOISOTOPES, BETA-MINUS DECAY RADIOISOTOPES, CESIUM ISOTOPES, EASTERN EUROPE, ENVIRONMENTAL TRANSPORT, EUROPE, INTERMEDIATE MASS NUCLEI, ISOTOPES, MASS TRANSFER, MEASURING INSTRUMENTS, NUCLEI, ODD-EVEN NUCLEI, RADIATION DOSE DISTRIBUTIONS, RADIOISOTOPES, SPECTROMETERS, YEARS LIVING RADIOISOTOPES
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