[en] This paper analyzes the characteristics of alloy compositions with large hydrogen storage capacities in Laves phase-related body-centered cubic (bcc) solid solution alloy systems using the cluster line approach. Since a dense-packed icosahedral cluster A₆B₇ characterizes the local structure of AB₂ Laves phases, in an A-B-C ternary system, such as Ti-Cr (Mn, Fe)-V, where A-B forms AB₂ Laves phases while A-C and B-C tend to form solid solutions, a cluster line A₆B₇-C is constructed by linking A₆B₇ to C. The alloy compositions with large hydrogen storage capacities are generally located near this line and are approximately expressed with the cluster-plus-glue-atom model. The cluster line alloys (Ti₆Cr₇)_100-xV_x (x = 2.5-70 at.%) exhibit different structures and hence different hydrogen storage capacities with increasing V content. The alloys (Ti₆Cr₇)₉₅V₅ and Ti₃₀Cr₄₀V₃₀ with bcc solid solution structure satisfy the cluster-plus-glue-atom model