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AbstractAbstract
[en] Strontium-90 is one of the most hazardous materials managed by agencies charged with protecting the public from radiation. Traditional radiometric methods have been limited by low sample throughput and slow turnaround times. Mass spectrometry offers the advantage of shorter analysis times and the ability to measure samples immediately after processing, however conventional mass spectrometric techniques are susceptible to molecular isobaric interferences that limit their overall sensitivity. In contrast, accelerator mass spectrometry is insensitive to molecular interferences and we have therefore begun developing a method for determination of 90Sr by accelerator mass spectrometry. Despite a pervasive interference from 90Zr, our initial development has yielded an instrumental background of ∼108 atoms (75 mBq) per sample. Further refinement of our system (e.g. redesign of our detector, use of alternative target materials) is expected to push the background below 106 atoms, close to the theoretical limit for AMS. Once we have refined our system and developed suitable sample preparation protocols, we will utilize our capability in applications to homeland security, environmental monitoring and human health
Primary Subject
Source
ECAART-9: 9. European conference on accelerators in applied research and technology; Florence (Italy); 3-7 Sep 2007; S0168-583X(08)00244-9; Available from http://dx.doi.org/10.1016/j.nimb.2008.03.088; Copyright (c) 2008 Elsevier Science B.V., Amsterdam, The Netherlands, All rights reserved.; Country of input: International Atomic Energy Agency (IAEA)
Record Type
Journal Article
Literature Type
Conference
Journal
Nuclear Instruments and Methods in Physics Research. Section B, Beam Interactions with Materials and Atoms; ISSN 0168-583X;
; CODEN NIMBEU; v. 266(10); p. 2242-2245

Country of publication
ALKALINE EARTH ISOTOPES, BETA DECAY RADIOISOTOPES, BETA-MINUS DECAY RADIOISOTOPES, EVEN-EVEN NUCLEI, INTERMEDIATE MASS NUCLEI, ISOMERIC TRANSITION ISOTOPES, ISOTOPES, MATERIALS, MILLISECONDS LIVING RADIOISOTOPES, NUCLEI, RADIOISOTOPES, SPECTROSCOPY, STABLE ISOTOPES, STRONTIUM ISOTOPES, YEARS LIVING RADIOISOTOPES, ZIRCONIUM ISOTOPES
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