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AbstractAbstract
[en] The pyrochlore slab (kagome bilayer) compounds SrCr9xGa12-9xO19 (SCGO; x<1) and Ba2Sn2ZnCr7xGa10-7xO22 (BSZCGO; x<1), are frustrated systems with quite similar magnetic properties of the spin S = 3/2 Cr3+ ions. Neutron scattering studies have shown that the two compounds have a completely dynamic magnetic response in a broad temperature range. In both systems the development of short-ranged dynamic correlations leads to a low-T state that can be understood as local clusters with antiferromagnetic character. At liquid He temperatures a partial freezing of the magnetic fluctuations is observed as an increase of the elastic resolved response. A large majority of the magnetic moments remain fluctuating and one also observes a low-energy (long-time) relaxation in the vicinity of the macroscopic freezing. Time and temperature dependence of this relaxation appear system dependent without critical behavior, and we conclude that the freezing is a consequence of the establishment of a coherent quantum state
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1 Apr 2007; vp; International Conference on Highly Frustrated Magnetism; Osaka (Japan); 15-19 Aug 2006; ORNL/PTS--5867; KC0204019; ERKCSNX; AC05-00OR22725; Available from Oak Ridge National Laboratory
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Miscellaneous
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Conference
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