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AbstractAbstract
[en] Elemental and isotopic ratio analyses of U ore concentrate samples, from the 3 operating U mining facilities in Australia, were carried out to determine if significant variations exist between their products, thereby allowing the U ore concentrate's origin to be identified. Elemental analyses were conducted using inductively coupled plasma mass spectrometry (ICP-MS) and X-ray fluorescence spectrometry (XRF). Lead isotope ratios were measured using ICP-MS and U isotope analyses were conducted using thermal ionisation mass spectrometry (TIMS). Minute quantities of sample, such as that obtained from a swipe, were also examined for elemental concentrations using secondary ion mass spectrometry (SIMS). The results of multivariate statistical analysis show clear patterns in the trace elemental composition of the processed U ores, indicating that it is possible to use this feature as a unique identifier of an Australian U ore concentrate's source. Secondary ion mass spectrometry analyses also allow individual particles to be differentiated using this 'fingerprinting' technique. Isotope ratios determined using TIMS reveal that there is a significant difference in the n(234U)/n(238U) isotope ratio between the U ore concentrate from each mine
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S0883-2927(07)00333-2; Available from http://dx.doi.org/10.1016/j.apgeochem.2007.12.004; Copyright (c) 2007 Elsevier Science B.V., Amsterdam, The Netherlands, All rights reserved.; Country of input: International Atomic Energy Agency (IAEA)
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ACTINIDE NUCLEI, ALPHA DECAY RADIOISOTOPES, CHEMICAL ANALYSIS, DIMENSIONLESS NUMBERS, ELECTROMAGNETIC RADIATION, EMISSION SPECTROSCOPY, EVEN-EVEN NUCLEI, HEAVY ION DECAY RADIOISOTOPES, HEAVY NUCLEI, IONIZING RADIATIONS, ISOTOPES, MAGNESIUM 28 DECAY RADIOISOTOPES, MASS SPECTROSCOPY, MATHEMATICS, MICROANALYSIS, NEON 24 DECAY RADIOISOTOPES, NONDESTRUCTIVE ANALYSIS, NUCLEI, ORES, RADIATIONS, RADIOISOTOPES, SPECTROSCOPY, SPONTANEOUS FISSION RADIOISOTOPES, STATISTICS, UNDERGROUND FACILITIES, URANIUM ISOTOPES, X-RAY EMISSION ANALYSIS, YEARS LIVING RADIOISOTOPES
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